Reisman, Sarah

Article from CaltechAUTHORS

• Chen, Li-Ming and Reisman, Sarah E. (2024) Enantioselective C(sp²)–C(sp³) Bond Construction by Ni Catalysis; Accounts of Chemical Research; Vol. 57; No. 5; 751-762; 10.1021/acs.accounts.3c00775
• Gao, Yang and Jiang, Baiyang, et el. (2024) Electrocatalytic Asymmetric Nozaki–Hiyama–Kishi Decarboxylative Coupling: Scope, Applications, and Mechanism; Journal of the American Chemical Society; Vol. 146; No. 7; 4872-4882; 10.1021/jacs.3c13442
• Raghavan, Priyanka and Haas, Brittany C., et el. (2023) Dataset Design for Building Models of Chemical Reactivity; ACS Central Science; PMCID PMC10755851; 10.1021/acscentsci.3c01163
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• Grünenfelder, Denise C. and Reisman, Sarah E., et el. (2023) Isolation, biosynthesis, and chemical syntheses of the hasubanan and acutumine alkaloids: A historical perspective; Tetrahedron; 133709; 10.1016/j.tet.2023.133709
• McNicholas, Brendon J. and Tong, Z. Jaron, et el. (2023) Electronic Structures of Nickel(II)-Bis(indanyloxazoline)-dihalide Catalysts: Understanding Ligand Field Contributions That Promote C(sp²)–C(sp³) Cross-Coupling; Inorganic Chemistry; Vol. 62; No. 34; 14010-14027; PMCID PMC10530056; 10.1021/acs.inorgchem.3c02048
• Turro, Raymond F. and Wahlman, Julie L. H., et el. (2023) Mechanistic Investigation of Ni-Catalyzed Reductive Cross-Coupling of Alkenyl and Benzyl Electrophiles; Journal of the American Chemical Society; Vol. 145; No. 27; 14705-14715; PMCID PMC10347553; 10.1021/jacs.3c02649
• Barbor, Jay P. and Nair, Vaishnavi N., et el. (2023) Development of a Nickel-Catalyzed N–N Coupling for the Synthesis of Hydrazides; Journal of the American Chemical Society; Vol. 145; No. 28; 15071-15077; PMCID PMC10360072; 10.1021/jacs.3c04834
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• Lacker, Caitlin R. and DeLano, Travis J., et el. (2022) Enantioselective Synthesis of N-Benzylic Heterocycles by Ni/Photoredox Dual Catalysis; Journal of the American Chemical Society; Vol. 144; No. 44; 20190-20195; PMCID PMC10326726; 10.1021/jacs.2c07917
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• Mendoza, Skyler D. and Rombola, Michael, et el. (2022) Expanding the Chiral Monoterpene Pool: Enantioselective Diels–Alder Reactions of α-Acyloxy Enones; Organic Letters; Vol. 24; No. 21; 3802-3806; 10.1021/acs.orglett.2c01343
• Gnaim, Samer and Bauer, Adriano, et el. (2022) Cobalt-electrocatalytic HAT for functionalization of unsaturated C–C bonds; Nature; Vol. 605; No. 7911; 687-695; PMCID PMC9206406; 10.1038/s41586-022-04595-3
• Holman, Karli R. and Stanko, Allison M., et el. (2022) Synthesis of Noraugustamine and Development of an Oxidative Heck/Aza-Wacker Cascade Cyclization; Organic Letters; Vol. 24; No. 16; 3019-3023; 10.1021/acs.orglett.2c00948
• Grünenfelder, Denise C. and Navarro, Raul, et el. (2022) Enantioselective Synthesis of (−)-10-Hydroxyacutuminine; Angewandte Chemie International Edition; Vol. 61; No. 16; Art. No. e202117480; 10.1002/anie.202117480
• Dibrell, Sara E. and Holman, Karli R., et el. (2022) Plugging the Leak: Empowering Women in Organic Chemistry; Angewandte Chemie International Edition; Vol. 61; No. 5; Art. No. e202111765; 10.1002/anie.202111765
• Wong, Alice R. and Fastuca, Nicholas J., et el. (2021) Total Syntheses of the C₁₉ Diterpenoid Alkaloids (–)-Talatisamine, (–)-Liljestrandisine, and (–)-Liljestrandinine by a Fragment Coupling Approach; ACS Central Science; Vol. 7; No. 8; 1311-1316; PMCID PMC8393236; 10.1021/acscentsci.1c00540
• Holman, K. R. and Stanko, A. M., et el. (2021) Palladium-catalyzed cascade cyclizations involving C–C and C–X bond formation: strategic applications in natural product synthesis; Chemical Society Reviews; Vol. 50; No. 14; 7891-7908; 10.1039/d0cs01385d
• Gao, Yang and Hill, David E., et el. (2021) Electrochemical Nozaki–Hiyama–Kishi Coupling: Scope, Applications, and Mechanism; Journal of the American Chemical Society; Vol. 143; No. 25; 9478-9488; PMCID PMC8720499; 10.1021/jacs.1c03007
• DeLano, Travis J. and Dibrell, Sara E., et el. (2021) Nickel-catalyzed asymmetric reductive cross-coupling of α-chloroesters with (hetero)aryl iodides; Chemical Science; Vol. 12; No. 22; 7758-7762; PMCID PMC8188512; 10.1039/d1sc00822f
• Reisman, Sarah E. and Maimone, Thomas J. (2021) Total Synthesis of Complex Natural Products: More Than a Race for Molecular Summits; Accounts of Chemical Research; Vol. 54; No. 8; 1815-1816; 10.1021/acs.accounts.1c00184
• Nakayama, Yasuaki and Maser, Michael R., et el. (2021) Total Synthesis of Ritterazine B; Journal of the American Chemical Society; Vol. 143; No. 11; 4187-4192; 10.1021/jacs.1c01372
• Dibrell, Sara E. and Tao, Yujia, et el. (2021) Synthesis of Complex Diterpenes: Strategies Guided by Oxidation Pattern Analysis; Accounts of Chemical Research; Vol. 54; No. 6; 1360-1373; PMCID PMC9169581; 10.1021/acs.accounts.0c00858
• Maser, Michael R. and Cui, Alexander Y., et el. (2021) Multilabel Classification Models for the Prediction of Cross-Coupling Reaction Conditions; Journal of Chemical Information and Modeling; Vol. 61; No. 1; 156-166; 10.1021/acs.jcim.0c01234
• Cowper, Nicholas G. W. and Hesse, Matthew J., et el. (2020) A copper-catalyzed asymmetric oxime propargylation enables the synthesis of the gliovirin tetrahydro-1,2-oxazine core; Chemical Science; Vol. 11; No. 43; 11897-11901; PMCID PMC8162951; 10.1039/d0sc04802j
• Blom, Annet E. M. and Su, Justin Y., et el. (2020) Synthesis and Biological Evaluation of Pyrroloindolines as Positive Allosteric Modulators of the α1β2γ2 GABA_A Receptor; ACS Medicinal Chemistry Letters; Vol. 11; No. 11; 2204-2211; PMCID PMC7667864; 10.1021/acsmedchemlett.0c00340
• Fastuca, Nicholas J. and Wong, Alice R., et el. (2020) Asymmetric Michael Addition of Dimethyl Malonate to 2 Cyclopenten-1-one Catalyzed by a Heterobimetallic Complex; Organic Syntheses; Vol. 97; 327-338; PMCID PMC9128456; 10.15227/orgsyn.097.0327
• Reisman, Sarah E. and Sarpong, Richmond, et el. (2020) Organic Chemistry: A Call to Action for Diversity and Inclusion; ACS Central Science; Vol. 6; No. 8; 1241-1247; PMCID PMC7453412; 10.1021/acscentsci.0c01027
• Reisman, Sarah E. and Sarpong, Richmond, et el. (2020) Organic Chemistry: A Call to Action for Diversity and Inclusion; Organometallics; Vol. 39; No. 16; 2931-2936; 10.1021/acs.organomet.0c00519
• Reisman, Sarah E. and Sarpong, Richmond, et el. (2020) Organic Chemistry: A Call to Action for Diversity and Inclusion; Journal of Organic Chemistry; Vol. 85; No. 16; 10287-10292; 10.1021/acs.joc.0c01607
• Reisman, Sarah E. and Sarpong, Richmond, et el. (2020) Organic Chemistry: A Call to Action for Diversity and Inclusion; Organic Letters; Vol. 22; No. 16; 6223-6228; 10.1021/acs.orglett.0c02559
• Hofstra, Julie L. and DeLano, Travis J., et el. (2020) Synthesis of Chiral Bisoxazoline Ligands: (3aR,3a'R,8aS,8a'S)-2,2'-(cyclopropane-1,1-diyl)bis(3a,8a-dihydro-8H-indeno[1,2-d]oxazole); Organic Syntheses; Vol. 97; 172-188; PMCID PMC8294164; 10.15227/orgsyn.097.0172
• Poremba, Kelsey E. and Dibrell, Sara E., et el. (2020) Nickel-Catalyzed Enantioselective Reductive Cross-Coupling Reactions; ACS Catalysis; Vol. 10; No. 15; 8237-8246; PMCID PMC7470226; 10.1021/acscatal.0c01842
• Wittmann, Bruce J. and Knight, Anders M., et el. (2020) Diversity-Oriented Enzymatic Synthesis of Cyclopropane Building Blocks; ACS Catalysis; Vol. 10; No. 13; 7112-7116; PMCID PMC7709968; 10.1021/acscatal.0c01888
• Dibrell, Sara E. and Maser, Michael R., et el. (2020) SeO₂-Mediated Oxidative Transposition of Pauson–Khand Products; Journal of the American Chemical Society; Vol. 142; No. 14; 6483-6487; 10.1021/jacs.9b13818
• Hofstra, Julie L. and Poremba, Kelsey E., et el. (2019) Nickel-Catalyzed Conversion of Enol Triflates into Alkenyl Halides; Angewandte Chemie International Edition; Vol. 58; No. 42; 14901-14905; PMCID PMC7179072; 10.1002/anie.201906815
• Han, Arthur and Tao, Yujia, et el. (2019) A 16-step synthesis of the isoryanodane diterpene (+)-perseanol; Nature; Vol. 573; No. 7775; 563-567; PMCID PMC7123484; 10.1038/s41586-019-1580-x
• DeLano, Travis J. and Reisman, Sarah E. (2019) Enantioselective Electroreductive Coupling of Alkenyl and Benzyl Halides via Nickel Catalysis; ACS Catalysis; Vol. 9; No. 8; 6751-6754; PMCID PMC7190267; 10.1021/acscatal.9b01785
• Beck, Jordan C. and Lacker, Caitlin R., et el. (2019) A modular approach to prepare enantioenriched cyclobutanes: synthesis of (+)-rumphellaone A; Chemical Science; Vol. 10; No. 8; 2315-2319; PMCID PMC6385545; 10.1039/c8sc05444d
• Carreira, Erick M. and Brimble, Margaret, et el. (2019) Organic Letters 2.0: A New Beginning; Organic Letters; Vol. 21; No. 1; 1-4; 10.1021/acs.orglett.8b03964
• Su, Justin Y. and Grünenfelder, Denise C., et el. (2018) Radical Deoxychlorination of Cesium Oxalates for the Synthesis of Alkyl Chlorides; Organic Letters; Vol. 20; No. 16; 4912-4916; 10.1021/acs.orglett.8b02045
• Xu, Chen and Han, Arthur, et el. (2018) An Oxidative Dearomatization Approach To Prepare the Pentacyclic Core of Ryanodol; Organic Letters; Vol. 20; No. 13; 3793-3796; PMCID PMC6103443; 10.1021/acs.orglett.8b01387
• Chapman, Lauren M. and Beck, Jordan C., et el. (2018) Evolution of a Strategy for the Enantioselective Total Synthesis of (+)-Psiguadial B; Journal of Organic Chemistry; Vol. 83; No. 11; 6066-6085; PMCID PMC5990278; 10.1021/acs.joc.8b00728
• Farney, Elliot P. and Feng, Sean S., et el. (2018) Total Synthesis of (+)-Pleuromutilin; Journal of the American Chemical Society; Vol. 140; No. 4; 1267-1270; PMCID PMC5988231; 10.1021/jacs.7b13260
• Hofstra, Julie L. and Cherney, Alan H., et el. (2018) Synthesis of Enantioenriched Allylic Silanes via Nickel-Catalyzed Reductive Cross-Coupling; Journal of the American Chemical Society; Vol. 140; No. 1; 139-142; PMCID PMC5851001; 10.1021/jacs.7b11707
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• Poremba, Kelsey E. and Kadunce, Nathaniel T., et el. (2017) Nickel-Catalyzed Asymmetric Reductive Cross-Coupling To Access 1,1-Diarylalkanes; Journal of the American Chemical Society; Vol. 139; No. 16; 5684-5687; PMCID PMC5851002; 10.1021/jacs.7b01705
• Suzuki, Naoyuki and Hofstra, Julie L., et el. (2017) Nickel-Catalyzed Enantioselective Cross-Coupling of N-Hydroxyphthalimide Esters with Vinyl Bromides; Organic Letters; Vol. 19; No. 8; 2150-2153; PMCID PMC5868419; 10.1021/acs.orglett.7b00793
• Wang, Haoxuan and Regan, Clinton J., et el. (2017) Enantioselective Synthesis of (−)-Acetylapoaranotin; Organic Letters; Vol. 19; No. 7; 1698-1701; PMCID PMC5387676; 10.1021/acs.orglett.7b00418
• Chuang, Kangway V. and Kieffer, Madeleine E., et el. (2016) A Mild and General Larock Indolization Protocol for the Preparation of Unnatural Tryptophans; Organic Letters; Vol. 18; No. 18; 4750-4753; PMCID PMC5505074; 10.1021/acs.orglett.6b02477
• Chuang, Kangway V. and Xu, Chen, et el. (2016) A 15-step synthesis of (+)-ryanodol; Science; Vol. 353; No. 6302; 912-915; PMCID PMC5505075; 10.1126/science.aag1028
• Chapman, Lauren M. and Beck, Jordan C., et el. (2016) Enantioselective Total Synthesis of (+)-Psiguadial B; Journal of the American Chemical Society; Vol. 138; No. 31; 9803-9806; 10.1021/jacs.6b07229
• Daniels, Blake E. and Ni, Jane, et el. (2016) Synthesis of Enantioenriched Indolines by a Conjugate Addition/Asymmetric Protonation/Aza-Prins Cascade Reaction; Angewandte Chemie International Edition; Vol. 55; No. 10; 3398-3402; PMCID PMC4843768; 10.1002/anie.201510972
• Cherney, Alan H. and Kadunce, Nathaniel T., et el. (2015) Enantioselective and Enantiospecific Transition-Metal-Catalyzed Cross-Coupling Reactions of Organometallic Reagents To Construct C–C Bonds; Chemical Reviews; Vol. 115; No. 17; 9587-9652; PMCID PMC4566132; 10.1021/acs.chemrev.5b00162
• Kadunce, Nathaniel T. and Reisman, Sarah E. (2015) Nickel-Catalyzed Asymmetric Reductive Cross-Coupling between Heteroaryl Iodides and α-Chloronitriles; Journal of the American Chemical Society; Vol. 137; No. 33; 10480-10483; PMCID PMC5066588; 10.1021/jacs.5b06466
• Jang, Kyoung-Soon and Nani, Roger R., et el. (2015) A cationic cysteine-hydrazide as an enrichment tool for the mass spectrometric characterization of bacterial free oligosaccharides; Analytical and Bioanalytical Chemistry; Vol. 407; No. 20; 6181-6190; PMCID PMC4539134; 10.1007/s00216-015-8798-8
• Reisman, Sarah E. (2015) From alkaloids to terpenoids: New strategies and tactics for the synthesis of polycyclic natural products; Abstracts of Papers of the American Chemical Society; Vol. 249; ORGN-219
• Cherney, Alan H. and Reisman, Sarah E. (2014) Nickel-Catalyzed Asymmetric Reductive Cross-Coupling Between Vinyl and Benzyl Electrophiles; Journal of the American Chemical Society; Vol. 136; No. 41; 14365-14368; PMCID PMC4210114; 10.1021/ja508067c
• Yeoman, John T. S. and Cha, Jacob Y., et el. (2014) A unified strategy for the synthesis of (−)-maoecrystal Z, (−)-trichorabdal A, and (−)-longikaurin E; Tetrahedron; Vol. 70; No. 27-28; 4070-4088; 10.1016/j.tet.2014.03.071
• Wang, Haoxuan and Reisman, Sarah E. (2014) Enantioselective Total Synthesis of (-)-Lansai B and (+)-Nocardioazines A and B; Angewandte Chemie International Edition; Vol. 53; No. 24; 6206-6210; PMCID PMC4086423; 10.1002/anie.201402571
• Cherney, Alan H. and Reisman, Sarah E. (2014) Pd-catalyzed Fukuyama cross-coupling of secondary organozinc reagents for the direct synthesis of unsymmetrical ketones; Tetrahedron; Vol. 70; No. 20; 3259-3265; 10.1016/j.tet.2013.11.104
• Repka, Lindsay M. and Reisman, Sarah E. (2013) Recent Developments in the Catalytic, Asymmetric Construction of Pyrroloindolines Bearing All-Carbon Quaternary Stereocenters; Journal of Organic Chemistry; Vol. 78; No. 24; 12314-12320; PMCID PMC3905788; 10.1021/jo4017953
• Hsiao, Elaine Y. and McBride, Sara W., et el. (2013) Microbiota Modulate Behavioral and Physiological Abnormalities Associated with Neurodevelopmental Disorders; Cell; Vol. 155; No. 7; 1451-1463; PMCID PMC3897394; 10.1016/j.cell.2013.11.024
• Yeoman, John T. S. and Mak, Victor W., et el. (2013) A Unified Strategy to ent-Kauranoid Natural Products: Total Syntheses of (−)-Trichorabdal A and (−)-Longikaurin E; Journal of the American Chemical Society; Vol. 135; No. 32; 11764-11767; 10.1021/ja406599a
• Wang, Jane Ni Haoxuan and Reisman, Sarah E. (2013) Direct, enantioselective synthesis of pyrroloindolines and indolines from simple indole derivatives; Tetrahedron; Vol. 69; No. 27-28; 5622-5633; PMCID PMC3769991; 10.1016/j.tet.2013.04.003
• Cherney, Alan H. and Kadunce, Nathaniel T., et el. (2013) Catalytic Asymmetric Reductive Acyl Cross-Coupling: Synthesis of Enantioenriched Acyclic α,α-Disubstituted Ketones; Journal of the American Chemical Society; Vol. 135; No. 20; 7442-7445; 10.1021/ja402922w
• Nani, Roger R. and Reisman, Sarah E. (2013) α-Diazo-β-ketonitriles: Uniquely Reactive Substrates for Arene and Alkene Cyclopropanation; Journal of the American Chemical Society; Vol. 135; No. 19; 7304-7311; 10.1021/ja401610p
• Kieffer, Madeleine E. and Chuang, Kangway V., et el. (2013) Copper-Catalyzed Diastereoselective Arylation of Tryptophan Derivatives: Total Synthesis of (+)-Naseseazines A and B; Journal of the American Chemical Society; Vol. 135; No. 15; 5557-5560; PMCID PMC3662218; 10.1021/ja4023557
• Codelli, Julian A. and Reisman, Sarah E. (2013) Pactamycin Made Easy; Science; Vol. 340; No. 6129; 152-153; 10.1126/science.1236882
• Lim, Andrew D. and Codelli, Julian A., et el. (2012) Catalytic asymmetric synthesis of highly substituted pyrrolizidines; Chemical Science; Vol. 4; No. 2; 650-654; PMCID PMC3614418; 10.1039/c2sc21617e
• Kieffer, Madeleine E. and Chuang, Kangway V., et el. (2012) A copper-catalyzed arylation of tryptamines for the direct synthesis of aryl pyrroloindolines; Chemical Science; Vol. 3; No. 11; 3170-3174; PMCID PMC3480223; 10.1039/c2sc20914d
• Yeoman, John T. S. and Reisman, Sarah E. (2012) Single molecules put a ring on it; Nature; Vol. 490; No. 7419; 179-180; 10.1038/490179a
• Navarro, Raul and Reisman, Sarah E. (2012) Rapid Construction of the Aza-Propellane Core of Acutumine via a Photochemical [2 + 2] Cycloaddition Reaction; Organic Letters; Vol. 14; No. 17; 4354-4357; PMCID PMC3445413; 10.1021/ol3017963
• Kieffer, Madeleine E. and Repka, Lindsay M., et el. (2012) Enantioselective Synthesis of Tryptophan Derivatives by a Tandem Friedel–Crafts Conjugate Addition/Asymmetric Protonation Reaction; Journal of the American Chemical Society; Vol. 134; No. 11; 5131-5137; PMCID PMC3310256; 10.1021/ja209390d
• Codelli, Julian A. and Puchlopek, Angela L. A., et el. (2012) Enantioselective Total Synthesis of (—)-Acetylaranotin, a Dihydrooxepine Epidithiodiketopiperazine; Journal of the American Chemical Society; Vol. 134; No. 4; 1930-1933; PMCID PMC3271125; 10.1021/ja209354e
• Reisman, Sarah E. and Nani, Roger R., et el. (2011) Buchner and Beyond: Arene Cyclopropanation as Applied to Natural Product Total Synthesis; Synlett; Vol. 2011; No. 17; 2437-2442; 10.1055/s-0031-1289520
• Cha, Jacob Y. and Yeoman, John T. S., et el. (2011) A Concise Total Synthesis of (--)-Maoecrystal Z; Journal of the American Chemical Society; Vol. 133; No. 38; 14964-14967; 10.1021/ja2073356
• Chuang, Kangway V. and Navarro, Raul, et el. (2011) Short, Enantioselective Total Syntheses of (—)-8-Demethoxyrunanine and (—)-Cepharatines A, C, and D; Angewandte Chemie International Edition; Vol. 50; No. 40; 9447-9451; PMCID PMC3520487; 10.1002/anie.201104487
• Reisman, Sarah E. (2011) Medicinal chemistry: New lead for pain treatment; Nature; Vol. 473; No. 7348; 458-459; 10.1038/473458a
• Chuang, Kangway V. and Navarro, Raul, et el. (2011) Benzoquinone-derived sulfinyl imines as versatile intermediates for alkaloid synthesis: Total synthesis of (–)-3-demethoxyerythratidinone; Chemical Science; Vol. 2; No. 6; 1086-1089; 10.1039/C1SC00095K
• Levin, Sergiy and Nani, Roger R., et el. (2011) Enantioselective Total Synthesis of (+)-Salvileucalin B; Journal of the American Chemical Society; Vol. 133; No. 4; 774-776; 10.1021/ja110192b
• Repka, Lindsay M. and Ni, Jane, et el. (2010) Enantioselective Synthesis of Pyrroloindolines by a Formal [3 + 2] Cycloaddition Reaction; Journal of the American Chemical Society; Vol. 132; No. 41; 14418-14420; PMCID PMC3222144; 10.1021/ja107328g
• Freeman, David B. and Holubec, Alexandra A., et el. (2010) Welwitindolinone C synthetic studies. Construction of the welwitindolinone carbon skeleton via a transannular nitrone cycloaddition; Tetrahedron; Vol. 66; No. 33; 6647-6655; PMCID PMC2924776; 10.1016/j.tet.2010.04.131
• Levin, Sergiy and Nani, Roger R., et el. (2010) Rapid Assembly of the Salvileucalin B Norcaradiene Core; Organic Letters; Vol. 12; No. 4; 780-783; 10.1021/ol902848k
• Reisman, Sarah E. and Doyle, Abigail G., et el. (2008) Enantioselective Thiourea-Catalyzed Additions to Oxocarbenium Ions; Journal of the American Chemical Society; Vol. 130; No. 23; 7198-7199; PMCID PMC2574628; 10.1021/ja801514m
• Reisman, Sarah E. and Ready, Joseph M., et el. (2008) Evolution of a Synthetic Strategy: Total Synthesis of (±)-Welwitindolinone A Isonitrile; Journal of the American Chemical Society; Vol. 130; No. 6; 2087-2100; 10.1021/ja076663z
• Reisman, Sarah E. and Ready, Joseph M., et el. (2006) Total Synthesis of (±)-Welwitindolinone A Isonitrile; Journal of the American Chemical Society; Vol. 128; No. 5; 1448-1449; 10.1021/ja057640s
• Ready, Joseph M. and Reisman, Sarah E., et el. (2004) A Mild and Efficient Synthesis of Oxindoles: Progress Towards the Synthesis of Welwitindolinone A Isonitrile; Angewandte Chemie International Edition; Vol. 43; No. 10; 1270-1272; 10.1002/anie.200353282
• Ovaska, Timo V. and Reisman, Sarah E., et el. (2001) Facile Entry to the Tetracyclic 5-7-6-3 Tigliane Ring System; Organic Letters; Vol. 3; No. 1; 115-117; 10.1021/ol006823a